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Supplement containing data related to the 2021 Global Carbon Budget from the Global Carbon Project. The original article is Friedlingstein et al: Global Carbon Budget 2021, Earth Syst. Sci. Data Discussions, 2021. https://doi.org/10.5194/essd-xx-xxxx-2021. Further information is available on: http://www.globalcarbonproject.org/carbonbudget. File Global_Carbon_Budget_2021v1.0.xlsx includes the following: 1. Summary 2. Global Carbon Budget 3. Fossil fuel emissions by Fuel Type 4. Land-use change emissions 5. Ocean Sink 6. Terrestrial sink 7. Historical Budget. File National_Carbon_Emissions_2020v1.0.xlsx includes the following: 1. Summary 2. Territorial emissions 3. Consumption emissions 4. Emissions transfers 5. Country definitions 6. Disaggregation 7. Aggregation